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Full Record Details
Persistent URL
http://purl.org/net/epubs/work/65739
Record Status
Checked
Record Id
65739
Title
Probing Chemistry and Kinetics of Reactions in Heterogeneous Catalysts
Contributors
T Youngs
,
H Manyar
,
DT Bowron (STFC Rutherford Appleton Lab.)
,
LF Gladden
,
C Hardacre
Abstract
Using benzene hydrogenation over Pt/SiO2 as an industrially-relevant example, we show that state-of-the-art neutron total scattering methods spanning a wide Q-range now permit relevant time-resolved catalytic chemistry to be probed directly in situ. The method gives access to the reaction rates on both nanometric and atomic length scales, whilst simultaneously providing an atomistic structural viewpoint on the reaction mechanism itself.
Organisation
ISIS
,
ISIS-NIMROD
,
STFC
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Language
English (EN)
Type
Details
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Year
Journal Article
Chem Sci
4, no. 9 (2013): 3484-3489.
doi:10.1039/c3sc51477c
2013
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